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Organosulfur- and organoselenium-containing compounds play a crucial role in organic synthesis. These sulfur-containing molecules are widely applied in pharmaceuticals, materials, natural products, and food. Additionally, sulfur and selenium show divergent functions and potencies in different oxidative states, leading to the rich chemistry of their transformations. This Molecules Special Issue introduces organosulfur and organoselenium chemistry in fields such as organic synthesis, materials, chemical biology, and computational chemistry, and contains eleven articles and four reviews. This Special Issue will be useful to scientists, researchers, and graduate students in the fields of organic chemistry, materials chemistry, chemical biology, and computational chemistry. We thank our many prominent colleagues for their contributions.

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